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The geometries of the monometallic (Au 8 and Pd 8) and bimetallic clusters (Au 8-n Pd n ) are shown in Figure. Figure1. 1. As reported earlier, Au 8 has a planar structure and prefers to be in the singlet spin state, whereas the Pd 8 cluster possesses a three-dimensional structure with a triplet spin state. Carbohydrate dehydrogenation and O2 consumption feed reactions that effectively lower the spin quantum number (S) of O2 from 1 to 1/2 and finally to 0. Oxidase-catalyzed univalent reduction of O2 (S = 1; triplet multiplicity) yields hydrodioxylic acid (HO2) and its conjugate base superoxide, O2- (S = 1/2; doublet multiplicity).

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Analysis of differences in oxygen sensitivity of Fe-S clusters.

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